Tracing the sources of the different magnetic behavior in the two phases of the bistable (BDTA)2[Co(mnt)2] compound

Abstract

A complete computational study of the magnetic properties of the two known phases of the bistable (BDTA)2[Co(mnt)2] compound is presented. The origin of their different magnetic properties can be traced to a variation in the values of the g tensor, together with a hitherto unknown change in the JAB values and their magnetic topology.