2010-06-08T10:16:37Z
2010-06-08T10:16:37Z
2000
Using a density functional method, we investigate the properties of liquid 4He droplets doped with atoms (Ne and Xe) and molecules ( SF6 and hydrogen cyanide). We consider the case of droplets having a quantized vortex pinned to the dopant. A liquid-drop formula is proposed that accurately describes the total energy of the complex and allows one to extrapolate the density functional results to large N. For a given impurity, we find that the formation of a dopant+vortex+4HeN complex is energetically favored below a critical size Ncr. Our results support the possibility to observe quantized vortices in helium droplets by means of spectroscopic techniques.
Article
Published version
English
Líquids quàntics; Química quàntica; Macromolècules; Quantum fluids; Quantum chemistry; Macromolecules
American Physical Society
Reproducció digital del document publicat en format paper, proporcionada per APS i http://dx.doi.org/10.1103/PhysRevLett.85.1028
Physical Review Letters, 2000, vol. 85, núm. 5, p. 1028-1031
http://dx.doi.org/10.1103/PhysRevLett.85.1028
(c) American Physical Society, 2000