Simple activation by acid of latent Ru-NHC-based metathesis initiators bearing 8-quinolinolate co-ligands

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dc.contributor	Ministerio de Economía y Competitividad (Espanya)
dc.contributor.author	Wappel, Julia
dc.contributor.author	Fischer, Roland C.
dc.contributor.author	Cavallo, Luigi
dc.contributor.author	Slugovc, Christian
dc.contributor.author	Poater Teixidor, Albert
dc.date	2016-12-02T08:40:49Z
dc.date	2016-12-02T08:40:49Z
dc.date	2016-01-28
dc.identifier.citation	1860-5397
dc.identifier.citation	025565
dc.identifier.uri	http://hdl.handle.net/10256/13310
dc.format	application/pdf
dc.language.iso	eng
dc.publisher	Beilstein-Institut
dc.relation	http://dx.doi.org/10.3762/bjoc.12.17
dc.relation	MINECO/PE 2015-2018/CTQ2014-59832-JIN
dc.relation	Reproducció digital del document publicat a: http://dx.doi.org/10.3762/bjoc.12.17
dc.relation	Beilstein Journal of Organic Chemistry, 2016, vol. 12, p.154-165
dc.relation	Articles publicats (D-Q)
dc.relation	info:eu-repo/grantAgreement/EC/FP7/293900
dc.rights	Attribution 4.0 Spain
dc.rights	info:eu-repo/semantics/openAccess
dc.rights	http://creativecommons.org/licenses/by/4.0/es/
dc.subject	Metàtesi (Química)
dc.subject	Metathesis (Chemistry)
dc.subject	Polimerització
dc.subject	Polymerization
dc.subject	Catalitzadors
dc.subject	Catalysts
dc.title	Simple activation by acid of latent Ru-NHC-based metathesis initiators bearing 8-quinolinolate co-ligands
dc.type	info:eu-repo/semantics/article
dc.type	info:eu-repo/semantics/publishedVersion
dc.description.abstract	A straightforward synthesis utilizing the ring-opening metathesis polymerization (ROMP) reaction is described for acid-triggered N,O-chelating ruthenium-based pre-catalysts bearing one or two 8-quinolinolate ligands. The innovative pre-catalysts were tested regarding their behavior in ROMP and especially for their use in the synthesis of poly(dicyclopentadiene) (pDCPD). Bearing either the common phosphine leaving ligand in the first and second Grubbs olefin metathesis catalysts, or the Ru–O bond cleavage for the next Hoveyda-type catalysts, this work is a step forward towards the control of polymer functionalization and living or switchable polymerizations
dc.description.abstract	A.P. thanks the Spanish MINECO for a project CTQ2014-59832-JIN, and European Commission for a Career Integration Grant (CIG09-GA-2011-293900

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